A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water

Hiranuma N, Adachi K, Bell DM, Belosi F, Beydoun H, Bhaduri B, Bingemer H, Budke C, Clemen H-C, Conen F, Cory KM, et al. (2019)
ATMOSPHERIC CHEMISTRY AND PHYSICS 19(7): 4823-4849.

Zeitschriftenaufsatz | Veröffentlicht | Englisch
 
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Autor*in
Hiranuma, Naruki; Adachi, Kouji; Bell, David M.; Belosi, Franco; Beydoun, Hassan; Bhaduri, Bhaskar; Bingemer, Heinz; Budke, CarstenUniBi; Clemen, Hans-Christian; Conen, Franz; Cory, Kimberly M.; Curtius, Joachim
Alle
Abstract / Bemerkung
We present the laboratory results of immersion freezing efficiencies of cellulose particles at supercooled temperature (T) conditions. Three types of chemically homogeneous cellulose samples are used as surrogates that represent supermicron and submicron ice-nucleating plant structural polymers. These samples include microcrystalline cellulose (MCC), fibrous cellulose (FC) and nanocrystalline cellulose (NCC). Our immersion freezing dataset includes data from various ice nucleation measurement techniques available at 17 different institutions, including nine dry dispersion and 11 aqueous suspension techniques. With a total of 20 methods, we performed systematic accuracy and precision analysis of measurements from all 20 measurement techniques by evaluating T-binned (1 degrees C) data over a wide T range (-36 degrees C< T <-4 degrees C). Specifically, we intercompared the geometric surface area-based ice nucleation active surface site (INAS) density data derived from our measurements as a function of T, n(s,geo). (T). Additionally, we also compared the n(s,geo). (T) values and the freezing spectral slope parameter (Delta log. n(s,geo))/Delta 1T) from our measurements to previous literature results. Results show all three cellulose materials are reasonably ice active. The freezing efficiencies of NCC samples agree reasonably well, whereas the diversity for the other two samples spans similar to 10 degrees C. Despite given uncertainties within each instrument technique, the overall trend of the n(s,geo)(T) spectrum traced by the T-binned average of measurements suggests that predominantly supermicron-sized cellulose particles (MCC and FC) generally act as more efficient ice-nucleating particles (INPs) than NCC with about 1 order of magnitude higher n(s,geo) (T).
Erscheinungsjahr
2019
Zeitschriftentitel
ATMOSPHERIC CHEMISTRY AND PHYSICS
Band
19
Ausgabe
7
Seite(n)
4823-4849
ISSN
1680-7316
eISSN
1680-7324
Page URI
https://pub.uni-bielefeld.de/record/2935399

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Hiranuma N, Adachi K, Bell DM, et al. A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water. ATMOSPHERIC CHEMISTRY AND PHYSICS. 2019;19(7):4823-4849.
Hiranuma, N., Adachi, K., Bell, D. M., Belosi, F., Beydoun, H., Bhaduri, B., Bingemer, H., et al. (2019). A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water. ATMOSPHERIC CHEMISTRY AND PHYSICS, 19(7), 4823-4849. doi:10.5194/acp-19-4823-2019
Hiranuma, N., Adachi, K., Bell, D. M., Belosi, F., Beydoun, H., Bhaduri, B., Bingemer, H., Budke, C., Clemen, H. - C., Conen, F., et al. (2019). A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water. ATMOSPHERIC CHEMISTRY AND PHYSICS 19, 4823-4849.
Hiranuma, N., et al., 2019. A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water. ATMOSPHERIC CHEMISTRY AND PHYSICS, 19(7), p 4823-4849.
N. Hiranuma, et al., “A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water”, ATMOSPHERIC CHEMISTRY AND PHYSICS, vol. 19, 2019, pp. 4823-4849.
Hiranuma, N., Adachi, K., Bell, D.M., Belosi, F., Beydoun, H., Bhaduri, B., Bingemer, H., Budke, C., Clemen, H.-C., Conen, F., Cory, K.M., Curtius, J., DeMott, P.J., Eppers, O., Grawe, S., Hartmann, S., Hoffmann, N., Hoehler, K., Jantsch, E., Kiselev, A., Koop, T., Kulkarni, G., Mayer, A., Murakami, M., Murray, B.J., Nicosia, A., Petters, M.D., Piazza, M., Polen, M., Reicher, N., Rudich, Y., Saito, A., Santachiara, G., Schiebel, T., Schill, G.P., Schneider, J., Segev, L., Stopelli, E., Sullivan, R.C., Suski, K., Szakall, M., Tajiri, T., Taylor, H., Tobo, Y., Ullrich, R., Weber, D., Wex, H., Whale, T.F., Whiteside, C.L., Yamashita, K., Zelenyuk, A., Moehler, O.: A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water. ATMOSPHERIC CHEMISTRY AND PHYSICS. 19, 4823-4849 (2019).
Hiranuma, Naruki, Adachi, Kouji, Bell, David M., Belosi, Franco, Beydoun, Hassan, Bhaduri, Bhaskar, Bingemer, Heinz, Budke, Carsten, Clemen, Hans-Christian, Conen, Franz, Cory, Kimberly M., Curtius, Joachim, DeMott, Paul J., Eppers, Oliver, Grawe, Sarah, Hartmann, Susan, Hoffmann, Nadine, Hoehler, Kristina, Jantsch, Evelyn, Kiselev, Alexei, Koop, Thomas, Kulkarni, Gourihar, Mayer, Amelie, Murakami, Masataka, Murray, Benjamin J., Nicosia, Alessia, Petters, Markus D., Piazza, Matteo, Polen, Michael, Reicher, Naama, Rudich, Yinon, Saito, Atsushi, Santachiara, Gianni, Schiebel, Thea, Schill, Gregg P., Schneider, Johannes, Segev, Lior, Stopelli, Emiliano, Sullivan, Ryan C., Suski, Kaitlyn, Szakall, Miklos, Tajiri, Takuya, Taylor, Hans, Tobo, Yutaka, Ullrich, Romy, Weber, Daniel, Wex, Heike, Whale, Thomas F., Whiteside, Craig L., Yamashita, Katsuya, Zelenyuk, Alla, and Moehler, Ottmar. “A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water”. ATMOSPHERIC CHEMISTRY AND PHYSICS 19.7 (2019): 4823-4849.

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