Correlating Oxygen Evolution Catalysts Activity and Electronic Structure by a High-Throughput Investigation of Ni1-y-zFeyCrzOx
Schwanke C, Stein HS, Xi L, Sliozberg K, Schuhmann W, Ludwig A, Aziz-Lange K (2017)
SCIENTIFIC REPORTS 7(1): 44192.
Zeitschriftenaufsatz
| Veröffentlicht | Englisch
Download
Es wurden keine Dateien hochgeladen. Nur Publikationsnachweis!
Autor*in
Schwanke, Christoph;
Stein, Helge Soeren;
Xi, Lifei;
Sliozberg, Kirill;
Schuhmann, Wolfgang;
Ludwig, Alfred;
Aziz-Lange, KathrinUniBi
Einrichtung
Abstract / Bemerkung
High-throughput characterization by soft X-ray absorption spectroscopy (XAS) and electrochemical characterization is used to establish a correlation between electronic structure and catalytic activity of oxygen evolution reaction (OER) catalysts. As a model system a quasi-ternary materials library of Ni1-y-zFeyCrzOx was synthesized by combinatorial reactive magnetron sputtering, characterized by XAS, and an automated scanning droplet cell. The presence of Cr was found to increase the OER activity in the investigated compositional range. The electronic structure of Ni-II and Cr-III remains unchanged over the investigated composition spread. At the Fe L-edge a linear combination of two spectra was observed. These spectra were assigned to Fe-III in O-h symmetry and Fe-III in T-d symmetry. The ratio of Fe-III O-h to Fe-III T-d increases with the amount of Cr and a correlation between the presence of the Fe-III O-h and a high OER activity is found.
Erscheinungsjahr
2017
Zeitschriftentitel
SCIENTIFIC REPORTS
Band
7
Ausgabe
1
Art.-Nr.
44192
Urheberrecht / Lizenzen
ISSN
2045-2322
Page URI
https://pub.uni-bielefeld.de/record/2910497
Zitieren
Schwanke C, Stein HS, Xi L, et al. Correlating Oxygen Evolution Catalysts Activity and Electronic Structure by a High-Throughput Investigation of Ni1-y-zFeyCrzOx. SCIENTIFIC REPORTS. 2017;7(1): 44192.
Schwanke, C., Stein, H. S., Xi, L., Sliozberg, K., Schuhmann, W., Ludwig, A., & Aziz-Lange, K. (2017). Correlating Oxygen Evolution Catalysts Activity and Electronic Structure by a High-Throughput Investigation of Ni1-y-zFeyCrzOx. SCIENTIFIC REPORTS, 7(1), 44192. doi:10.1038/srep44192
Schwanke, Christoph, Stein, Helge Soeren, Xi, Lifei, Sliozberg, Kirill, Schuhmann, Wolfgang, Ludwig, Alfred, and Aziz-Lange, Kathrin. 2017. “Correlating Oxygen Evolution Catalysts Activity and Electronic Structure by a High-Throughput Investigation of Ni1-y-zFeyCrzOx”. SCIENTIFIC REPORTS 7 (1): 44192.
Schwanke, C., Stein, H. S., Xi, L., Sliozberg, K., Schuhmann, W., Ludwig, A., and Aziz-Lange, K. (2017). Correlating Oxygen Evolution Catalysts Activity and Electronic Structure by a High-Throughput Investigation of Ni1-y-zFeyCrzOx. SCIENTIFIC REPORTS 7:44192.
Schwanke, C., et al., 2017. Correlating Oxygen Evolution Catalysts Activity and Electronic Structure by a High-Throughput Investigation of Ni1-y-zFeyCrzOx. SCIENTIFIC REPORTS, 7(1): 44192.
C. Schwanke, et al., “Correlating Oxygen Evolution Catalysts Activity and Electronic Structure by a High-Throughput Investigation of Ni1-y-zFeyCrzOx”, SCIENTIFIC REPORTS, vol. 7, 2017, : 44192.
Schwanke, C., Stein, H.S., Xi, L., Sliozberg, K., Schuhmann, W., Ludwig, A., Aziz-Lange, K.: Correlating Oxygen Evolution Catalysts Activity and Electronic Structure by a High-Throughput Investigation of Ni1-y-zFeyCrzOx. SCIENTIFIC REPORTS. 7, : 44192 (2017).
Schwanke, Christoph, Stein, Helge Soeren, Xi, Lifei, Sliozberg, Kirill, Schuhmann, Wolfgang, Ludwig, Alfred, and Aziz-Lange, Kathrin. “Correlating Oxygen Evolution Catalysts Activity and Electronic Structure by a High-Throughput Investigation of Ni1-y-zFeyCrzOx”. SCIENTIFIC REPORTS 7.1 (2017): 44192.
Daten bereitgestellt von European Bioinformatics Institute (EBI)
1 Zitation in Europe PMC
Daten bereitgestellt von Europe PubMed Central.
Atomic-level insight into super-efficient electrocatalytic oxygen evolution on iron and vanadium co-doped nickel (oxy)hydroxide.
Jiang J, Sun F, Zhou S, Hu W, Zhang H, Dong J, Jiang Z, Zhao J, Li J, Yan W, Wang M., Nat Commun 9(1), 2018
PMID: 30038335
Jiang J, Sun F, Zhou S, Hu W, Zhang H, Dong J, Jiang Z, Zhao J, Li J, Yan W, Wang M., Nat Commun 9(1), 2018
PMID: 30038335
32 References
Daten bereitgestellt von Europe PubMed Central.
Chen, Energy Environ. Sci. 7(), 2014
Gong, Nano Res. 8(), 2014
Landon, ACS Catal. 2(), 2012
Li, ACS Catal. 4(), 2014
Singh, Electrochim. Acta 51(), 2006
Towards the computational design of solid catalysts.
Norskov JK, Bligaard T, Rossmeisl J, Christensen CH., Nat Chem 1(1), 2009
PMID: 21378799
Norskov JK, Bligaard T, Rossmeisl J, Christensen CH., Nat Chem 1(1), 2009
PMID: 21378799
Greeley, J. Phys. Chem. C 113(), 2009
Density functional theory in surface chemistry and catalysis.
Norskov JK, Abild-Pedersen F, Studt F, Bligaard T., Proc. Natl. Acad. Sci. U.S.A. 108(3), 2011
PMID: 21220337
Norskov JK, Abild-Pedersen F, Studt F, Bligaard T., Proc. Natl. Acad. Sci. U.S.A. 108(3), 2011
PMID: 21220337
Man, ChemCatChem 3(), 2011
Design principles for oxygen-reduction activity on perovskite oxide catalysts for fuel cells and metal-air batteries.
Suntivich J, Gasteiger HA, Yabuuchi N, Nakanishi H, Goodenough JB, Shao-Horn Y., Nat Chem 3(7), 2011
PMID: 21697876
Suntivich J, Gasteiger HA, Yabuuchi N, Nakanishi H, Goodenough JB, Shao-Horn Y., Nat Chem 3(7), 2011
PMID: 21697876
A perovskite oxide optimized for oxygen evolution catalysis from molecular orbital principles.
Suntivich J, May KJ, Gasteiger HA, Goodenough JB, Shao-Horn Y., Science 334(6061), 2011
PMID: 22033519
Suntivich J, May KJ, Gasteiger HA, Goodenough JB, Shao-Horn Y., Science 334(6061), 2011
PMID: 22033519
Calle-Vallejo, Chem. Sci. 4(), 2013
Hong, J. Phys. Chem. C 120(), 2016
An investigation of thin-film Ni-Fe oxide catalysts for the electrochemical evolution of oxygen.
Louie MW, Bell AT., J. Am. Chem. Soc. 135(33), 2013
PMID: 23859025
Louie MW, Bell AT., J. Am. Chem. Soc. 135(33), 2013
PMID: 23859025
Identification of highly active Fe sites in (Ni,Fe)OOH for electrocatalytic water splitting.
Friebel D, Louie MW, Bajdich M, Sanwald KE, Cai Y, Wise AM, Cheng MJ, Sokaras D, Weng TC, Alonso-Mori R, Davis RC, Bargar JR, Norskov JK, Nilsson A, Bell AT., J. Am. Chem. Soc. 137(3), 2015
PMID: 25562406
Friebel D, Louie MW, Bajdich M, Sanwald KE, Cai Y, Wise AM, Cheng MJ, Sokaras D, Weng TC, Alonso-Mori R, Davis RC, Bargar JR, Norskov JK, Nilsson A, Bell AT., J. Am. Chem. Soc. 137(3), 2015
PMID: 25562406
Bockris, J. Electrochem. Soc. 131(), 1984
Mechanistic studies of the oxygen evolution reaction by a cobalt-phosphate catalyst at neutral pH.
Surendranath Y, Kanan MW, Nocera DG., J. Am. Chem. Soc. 132(46), 2010
PMID: 20977209
Surendranath Y, Kanan MW, Nocera DG., J. Am. Chem. Soc. 132(46), 2010
PMID: 20977209
Electrochemical water oxidation with cobalt-based electrocatalysts from pH 0-14: the thermodynamic basis for catalyst structure, stability, and activity.
Gerken JB, McAlpin JG, Chen JY, Rigsby ML, Casey WH, Britt RD, Stahl SS., J. Am. Chem. Soc. 133(36), 2011
PMID: 21806043
Gerken JB, McAlpin JG, Chen JY, Rigsby ML, Casey WH, Britt RD, Stahl SS., J. Am. Chem. Soc. 133(36), 2011
PMID: 21806043
Bockris, J. Phys. Chem. 87(), 1983
Mechanistic studies of the oxygen evolution reaction mediated by a nickel-borate thin film electrocatalyst.
Bediako DK, Surendranath Y, Nocera DG., J. Am. Chem. Soc. 135(9), 2013
PMID: 23360238
Bediako DK, Surendranath Y, Nocera DG., J. Am. Chem. Soc. 135(9), 2013
PMID: 23360238
AUTHOR UNKNOWN, 0
van, Solid State Commun. 80(), 1991
Kendelewicz, Surf. Sci. 424(), 1999
Miedema, J. Electron Spectros. Relat. Phenomena 187(), 2013
1s2p resonant inelastic X-ray scattering of iron oxides.
de Groot FM, Glatzel P, Bergmann U, van Aken PA, Barrea RA, Klemme S, Havecker M, Knop-Gericke A, Heijboer WM, Weckhuysen BM., J Phys Chem B 109(44), 2005
PMID: 16853690
de Groot FM, Glatzel P, Bergmann U, van Aken PA, Barrea RA, Klemme S, Havecker M, Knop-Gericke A, Heijboer WM, Weckhuysen BM., J Phys Chem B 109(44), 2005
PMID: 16853690
New benchmark for water photooxidation by nanostructured alpha-Fe2O3 films.
Kay A, Cesar I, Gratzel M., J. Am. Chem. Soc. 128(49), 2006
PMID: 17147381
Kay A, Cesar I, Gratzel M., J. Am. Chem. Soc. 128(49), 2006
PMID: 17147381
Enabling unassisted solar water splitting by iron oxide and silicon.
Jang JW, Du C, Ye Y, Lin Y, Yao X, Thorne J, Liu E, McMahon G, Zhu J, Javey A, Guo J, Wang D., Nat Commun 6(), 2015
PMID: 26078190
Jang JW, Du C, Ye Y, Lin Y, Yao X, Thorne J, Liu E, McMahon G, Zhu J, Javey A, Guo J, Wang D., Nat Commun 6(), 2015
PMID: 26078190
Ludwig, Int. J. Mater. Res. 99(), 2008
Sliozberg, Chempluschem 80(), 2015
High-throughput screening of thin-film semiconductor material libraries II: characterization of Fe-W-O libraries.
Meyer R, Sliozberg K, Khare C, Schuhmann W, Ludwig A., ChemSusChem 8(7), 2015
PMID: 25727483
Meyer R, Sliozberg K, Khare C, Schuhmann W, Ludwig A., ChemSusChem 8(7), 2015
PMID: 25727483
Fe-Cr-Al containing oxide semiconductors as potential solar water-splitting materials.
Sliozberg K, Stein HS, Khare C, Parkinson BA, Ludwig A, Schuhmann W., ACS Appl Mater Interfaces 7(8), 2015
PMID: 25650842
Sliozberg K, Stein HS, Khare C, Parkinson BA, Ludwig A, Schuhmann W., ACS Appl Mater Interfaces 7(8), 2015
PMID: 25650842
High-throughput screening of thin-film semiconductor material libraries I: system development and case study for Ti-W-O.
Sliozberg K, Schafer D, Erichsen T, Meyer R, Khare C, Ludwig A, Schuhmann W., ChemSusChem 8(7), 2015
PMID: 25727402
Sliozberg K, Schafer D, Erichsen T, Meyer R, Khare C, Ludwig A, Schuhmann W., ChemSusChem 8(7), 2015
PMID: 25727402
Export
Markieren/ Markierung löschen
Markierte Publikationen
Web of Science
Dieser Datensatz im Web of Science®Quellen
PMID: 28287134
PubMed | Europe PMC
Suchen in
Google Scholar