Electron dynamics in a heterogeneous system: thin Ag films on Si(100)
Kennerknecht C, Dantscher S, Pfeiffer W, Autzen O, Wesenberg C, Hasselbrink E (2006)
Surface Science 600(18): 4269-4274.
Zeitschriftenaufsatz
| Veröffentlicht | Englisch
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Autor*in
Kennerknecht, Claudia;
Dantscher, Sandra;
Pfeiffer, WalterUniBi;
Autzen, Olaf;
Wesenberg, Claudia;
Hasselbrink, Eckart
Einrichtung
Abstract / Bemerkung
Photodesorption dynamics is strongly influenced by the electronic structure and electron dynamics of the substrate. Here we use time-resolved two-photon photoemission spectroscopy to investigate electron relaxation and transport in thin ultra-flat epitaxial Ag films on Si(I 00). Two-photon photoemission spectra obtained for excitation with 3.1 eV photons reveal that electron emission occurs preferentially from the Ag film. In contrast, the photoelectrons generated by two-photon excitation with 4.7 eV photons originate from the Si substrate. This conclusion is supported by intensity dependent spectral changes that can only be reconciled if both excitation steps occur in the Si substrate. In addition, this is corroborated by time-resolved experiments that reveal slow electron relaxation dynamics as it is expected for Si. Our results indicate that the excitation in the Si substrate and the transmission of electrons through the thin Ag film play an important role in electron dynamics in the heterogeneous system and can well be responsible for the film thickness and excitation wavelength dependence of photodesorption of NO2. (c) 2006 Elsevier B.V. All rights reserved.
Stichworte
charge transfer;
dynamics;
ultrafast;
heterogeneous system;
two-photon-photoemission;
thin films;
relaxation;
Ag(111);
Si(100)
Erscheinungsjahr
2006
Zeitschriftentitel
Surface Science
Band
600
Ausgabe
18
Seite(n)
4269-4274
ISSN
0039-6028
Page URI
https://pub.uni-bielefeld.de/record/2407627
Zitieren
Kennerknecht C, Dantscher S, Pfeiffer W, Autzen O, Wesenberg C, Hasselbrink E. Electron dynamics in a heterogeneous system: thin Ag films on Si(100). Surface Science. 2006;600(18):4269-4274.
Kennerknecht, C., Dantscher, S., Pfeiffer, W., Autzen, O., Wesenberg, C., & Hasselbrink, E. (2006). Electron dynamics in a heterogeneous system: thin Ag films on Si(100). Surface Science, 600(18), 4269-4274. https://doi.org/10.1016/j.susc.2006.02.072
Kennerknecht, Claudia, Dantscher, Sandra, Pfeiffer, Walter, Autzen, Olaf, Wesenberg, Claudia, and Hasselbrink, Eckart. 2006. “Electron dynamics in a heterogeneous system: thin Ag films on Si(100)”. Surface Science 600 (18): 4269-4274.
Kennerknecht, C., Dantscher, S., Pfeiffer, W., Autzen, O., Wesenberg, C., and Hasselbrink, E. (2006). Electron dynamics in a heterogeneous system: thin Ag films on Si(100). Surface Science 600, 4269-4274.
Kennerknecht, C., et al., 2006. Electron dynamics in a heterogeneous system: thin Ag films on Si(100). Surface Science, 600(18), p 4269-4274.
C. Kennerknecht, et al., “Electron dynamics in a heterogeneous system: thin Ag films on Si(100)”, Surface Science, vol. 600, 2006, pp. 4269-4274.
Kennerknecht, C., Dantscher, S., Pfeiffer, W., Autzen, O., Wesenberg, C., Hasselbrink, E.: Electron dynamics in a heterogeneous system: thin Ag films on Si(100). Surface Science. 600, 4269-4274 (2006).
Kennerknecht, Claudia, Dantscher, Sandra, Pfeiffer, Walter, Autzen, Olaf, Wesenberg, Claudia, and Hasselbrink, Eckart. “Electron dynamics in a heterogeneous system: thin Ag films on Si(100)”. Surface Science 600.18 (2006): 4269-4274.
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