Attosecond spectroscopy in condensed matter

Cavalieri AL, Müller N, Uphues T, Yakovlev VS, Baltuska A, Horvath B, Schmidt B, Blümel L, Holzwarth R, Hendel S, Drescher M, et al. (2007)
Nature 449(7165): 1029-1032.

Zeitschriftenaufsatz | Veröffentlicht | Englisch
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Cavalieri, A. L.; Müller, NorbertUniBi; Uphues, Thorsten; Yakovlev, V. S.; Baltuska, A.; Horvath, B.; Schmidt, B.; Blümel, L.; Holzwarth, R.; Hendel, StefanUniBi; Drescher, MarkusUniBi; Kleineberg, U.
Abstract / Bemerkung
Comprehensive knowledge of the dynamic behaviour of electrons in condensed-matter systems is pertinent to the development of many modern technologies, such as semiconductor and molecular electronics, optoelectronics, information processing and photo-voltaics. Yet it remains challenging to probe electronic processes, many of which take place in the attosecond (1 as = 10(-18) s) regime. In contrast, atomic motion occurs on the femtosecond (1 fs = 10(-15) s) timescale and has been mapped in solids in real time(1,2) using femtosecond X-ray sources(3). Here we extend the attosecond techniques(4,5) previously used to study isolated atoms in the gas phase to observe electron motion in condensed-matter systems and on surfaces in real time. We demonstrate our ability to obtain direct time-domain access to charge dynamics with attosecond resolution by probing photoelectron emission from single-crystal tungsten. Our data reveal a delay of approximately 100 attoseconds between the emission of photoelectrons that originate from localized core states of the metal, and those that are freed from delocalized conduction-band states. These results illustrate that attosecond metrology constitutes a powerful tool for exploring not only gas-phase systems, but also fundamental electronic processes occurring on the attosecond timescale in condensed-matter systems and on surfaces.
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Cavalieri AL, Müller N, Uphues T, et al. Attosecond spectroscopy in condensed matter. Nature. 2007;449(7165):1029-1032.
Cavalieri, A. L., Müller, N., Uphues, T., Yakovlev, V. S., Baltuska, A., Horvath, B., Schmidt, B., et al. (2007). Attosecond spectroscopy in condensed matter. Nature, 449(7165), 1029-1032.
Cavalieri, A. L., Müller, Norbert, Uphues, Thorsten, Yakovlev, V. S., Baltuska, A., Horvath, B., Schmidt, B., et al. 2007. “Attosecond spectroscopy in condensed matter”. Nature 449 (7165): 1029-1032.
Cavalieri, A. L., Müller, N., Uphues, T., Yakovlev, V. S., Baltuska, A., Horvath, B., Schmidt, B., Blümel, L., Holzwarth, R., Hendel, S., et al. (2007). Attosecond spectroscopy in condensed matter. Nature 449, 1029-1032.
Cavalieri, A.L., et al., 2007. Attosecond spectroscopy in condensed matter. Nature, 449(7165), p 1029-1032.
A.L. Cavalieri, et al., “Attosecond spectroscopy in condensed matter”, Nature, vol. 449, 2007, pp. 1029-1032.
Cavalieri, A.L., Müller, N., Uphues, T., Yakovlev, V.S., Baltuska, A., Horvath, B., Schmidt, B., Blümel, L., Holzwarth, R., Hendel, S., Drescher, M., Kleineberg, U., Echenique, P.M., Kienberger, R., Krausz, F., Heinzmann, U.: Attosecond spectroscopy in condensed matter. Nature. 449, 1029-1032 (2007).
Cavalieri, A. L., Müller, Norbert, Uphues, Thorsten, Yakovlev, V. S., Baltuska, A., Horvath, B., Schmidt, B., Blümel, L., Holzwarth, R., Hendel, Stefan, Drescher, Markus, Kleineberg, U., Echenique, P. M., Kienberger, R., Krausz, F., and Heinzmann, Ulrich. “Attosecond spectroscopy in condensed matter”. Nature 449.7165 (2007): 1029-1032.

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Fiess M, Schultze M, Goulielmakis E, Dennhardt B, Gagnon J, Hofstetter M, Kienberger R, Krausz F., Rev Sci Instrum 81(9), 2010
PMID: 20886972
Single-electron pulses for ultrafast diffraction.
Aidelsburger M, Kirchner FO, Krausz F, Baum P., Proc Natl Acad Sci U S A 107(46), 2010
PMID: 21041681
Determining the time zero for electronic dynamics.
Sansone G., Chemphyschem 11(17), 2010
PMID: 21053241
Tunable frequency-controlled isolated attosecond pulses characterized by either 750 nm or 400 nm wavelength streak fields.
Mashiko H, Bell MJ, Beck AR, Abel MJ, Nagel PM, Steiner CP, Robinson J, Neumark DM, Leone SR., Opt Express 18(25), 2010
PMID: 21164934
Attosecond photoelectron spectroscopy of metal surfaces.
Zhang CH, Thumm U., Phys Rev Lett 102(12), 2009
PMID: 19392274
Theoretical description of time-resolved photoemission spectroscopy: application to pump-probe experiments.
Freericks JK, Krishnamurthy HR, Pruschke T., Phys Rev Lett 102(13), 2009
PMID: 19392376
Measurement and optimization of isolated attosecond pulse contrast.
Pfeifer T, Abel MJ, Nagel PM, Boutu W, Bell MJ, Liu Y, Neumark DM, Leone SR., Opt Lett 34(12), 2009
PMID: 19529714
Optical detection of interfering pathways in subfemtosecond multielectron dynamics.
Zheltikov AM, Voronin AA, Kitzler M, Baltuska A, Ivanov M., Phys Rev Lett 103(3), 2009
PMID: 19659279
The development and applications of ultrafast electron nanocrystallography.
Ruan CY, Murooka Y, Raman RK, Murdick RA, Worhatch RJ, Pell A., Microsc Microanal 15(4), 2009
PMID: 19575833
The robustness of attosecond streaking measurements.
Gagnon J, Yakovlev VS., Opt Express 17(20), 2009
PMID: 19907553
Generating single attosecond pulse using multi-cycle lasers in a polarization gate.
Tosa V, Kovacs K, Altucci C, Velotta R., Opt Express 17(20), 2009
PMID: 19907555
Strong-field control and spectroscopy of attosecond electron-hole dynamics in molecules.
Smirnova O, Patchkovskii S, Mairesse Y, Dudovich N, Ivanov MY., Proc Natl Acad Sci U S A 106(39), 2009
PMID: 19805337
Generation of isolated attosecond pulses with 20 to 28 femtosecond lasers.
Feng X, Gilbertson S, Mashiko H, Wang H, Khan SD, Chini M, Wu Y, Zhao K, Chang Z., Phys Rev Lett 103(18), 2009
PMID: 19905806
Delay control in attosecond pump-probe experiments.
Chini M, Mashiko H, Wang H, Chen S, Yun C, Scott S, Gilbertson S, Chang Z., Opt Express 17(24), 2009
PMID: 19997386
Single-cycle nonlinear optics.
Goulielmakis E, Schultze M, Hofstetter M, Yakovlev VS, Gagnon J, Uiberacker M, Aquila AL, Gullikson EM, Attwood DT, Kienberger R, Krausz F, Kleineberg U., Science 320(5883), 2008
PMID: 18566281
Dynamic correlations with time-dependent quantum Monte Carlo.
Christov IP., J Chem Phys 128(24), 2008
PMID: 18601316
A tabletop femtosecond time-resolved soft x-ray transient absorption spectrometer.
Loh ZH, Khalil M, Correa RE, Leone SR., Rev Sci Instrum 79(7), 2008
PMID: 18681685
Direct measurement of core-level relaxation dynamics on a surface-adsorbate system.
Miaja-Avila L, Saathoff G, Mathias S, Yin J, La-o-vorakiat C, Bauer M, Aeschlimann M, Murnane MM, Kapteyn HC., Phys Rev Lett 101(4), 2008
PMID: 18764340
Intense few-cycle light pulses in the deep ultraviolet.
Graf U, Fiess M, Schultze M, Kienberger R, Krausz F, Goulielmakis E., Opt Express 16(23), 2008
PMID: 19581987
Attophysics: at a glance.
Villeneuve DM., Nature 449(7165), 2007
PMID: 17960231

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