PUB - Publikationen an der Universität Bielefeld

A newly developed "intense-field many-body S-matrix" theory (or IMST) for investigating highly nonperturbative interaction of strong laser pulses with many-electron atomic and molecular systems is briefly presented and the usefulness of the theory is demonstrated by direct calculations of (i) "hot electron plateaus" in ATI spectra of He, (ii) intensity dependence of double ionization yields of He, and (iii) multiple ionization yields of Xe, (iv) "enhanced ionization" of a diatomic molecule, H-2, and (v) of the polyatomic molecules benzene C6H6 and its cation C6H6+. The ATI spectra of He and the associated double ionization yields, as well as the multiple ionization yields of Xe, in the presence of intense femtosecond laser pulses, have been measured recently. The results of theoretical calculations are found to agree remarkably well with these experimental data. They confirm the crucial role of rescattering for the formation of the hot electron plateaus, and that of the "internal e-ne" process for the nonsequential double and multiple ionization of noble gases. The phenomenon of "enhanced ionization" at a specific internuclear distance for the diatomic molecular hydrogen, studied by previous authors, is confirmed and that for the polyatomic benzene molecule and its cation are predicted.