Attosecond metrology

Hentschel M, Kienberger R, Spielmann C, Reider GA, Milosevic N, Brabec T, Corkum P, Heinzmann U, Drescher M, Krausz F (2001)
NATURE 414(6863): 509-513.

Zeitschriftenaufsatz | Veröffentlicht | Englisch
 
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Autor*in
Hentschel, M; Kienberger, R; Spielmann, C; Reider, GA; Milosevic, N; Brabec, T; Corkum, P; Heinzmann, UlrichUniBi; Drescher, MarkusUniBi; Krausz, F
Abstract / Bemerkung
The generation of ultrashort pulses is a key to exploring the dynamic behaviour of matter on ever-shorter timescales. Recent developments have pushed the duration of laser pulses close to its natural limit-the wave cycle, which lasts somewhat longer than one femtosecond (1 fs = 10(-15) s) in the visible spectral range. Time-resolved measurements with these pulses are able to trace dynamics of molecular structure, but fail to capture electronic processes occurring on an attosecond (1 as = 10(-18) s) timescale. Here we trace electronic dynamics with a time resolution of less than or equal to 150 as by using a subfemtosecond soft-X-ray pulse and a few-cycle visible light pulse. Our measurement indicates an attosecond response of the atomic system, a soft-X-ray pulse duration of 650 +/- 150 as and an attosecond synchronism of the soft-X-ray pulse with the light field. The demonstrated experimental tools and techniques open the door to attosecond spectroscopy of bound electrons.
Erscheinungsjahr
2001
Zeitschriftentitel
NATURE
Band
414
Ausgabe
6863
Seite(n)
509-513
ISSN
0028-0836
Page URI
https://pub.uni-bielefeld.de/record/1615760

Zitieren

Hentschel M, Kienberger R, Spielmann C, et al. Attosecond metrology. NATURE. 2001;414(6863):509-513.
Hentschel, M., Kienberger, R., Spielmann, C., Reider, G. A., Milosevic, N., Brabec, T., Corkum, P., et al. (2001). Attosecond metrology. NATURE, 414(6863), 509-513. https://doi.org/10.1038/35107000
Hentschel, M, Kienberger, R, Spielmann, C, Reider, GA, Milosevic, N, Brabec, T, Corkum, P, Heinzmann, Ulrich, Drescher, Markus, and Krausz, F. 2001. “Attosecond metrology”. NATURE 414 (6863): 509-513.
Hentschel, M., Kienberger, R., Spielmann, C., Reider, G. A., Milosevic, N., Brabec, T., Corkum, P., Heinzmann, U., Drescher, M., and Krausz, F. (2001). Attosecond metrology. NATURE 414, 509-513.
Hentschel, M., et al., 2001. Attosecond metrology. NATURE, 414(6863), p 509-513.
M. Hentschel, et al., “Attosecond metrology”, NATURE, vol. 414, 2001, pp. 509-513.
Hentschel, M., Kienberger, R., Spielmann, C., Reider, G.A., Milosevic, N., Brabec, T., Corkum, P., Heinzmann, U., Drescher, M., Krausz, F.: Attosecond metrology. NATURE. 414, 509-513 (2001).
Hentschel, M, Kienberger, R, Spielmann, C, Reider, GA, Milosevic, N, Brabec, T, Corkum, P, Heinzmann, Ulrich, Drescher, Markus, and Krausz, F. “Attosecond metrology”. NATURE 414.6863 (2001): 509-513.

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Calibration of electron spectrometer resolution in attosecond streak camera.
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Thinner, smaller, faster: IR techniques to probe the functionality of biological and biomimetic systems.
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Determining the time zero for electronic dynamics.
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Monitoring and controlling the electron dynamics in helium with isolated attosecond pulses.
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Characterizing isolated attosecond pulses from hollow-core waveguides using multi-cycle driving pulses.
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Nuclear interference in the Coulomb explosion of H2+ in short vuv laser fields.
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Attosecond photoelectron spectroscopy of metal surfaces.
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Ultrafast probing of collective electron dynamics driven by dielectronic repulsion.
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Interferometry of attosecond pulse trains in the extreme ultraviolet wavelength region.
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Pulse compression of submillijoule few-optical-cycle infrared laser pulses using chirped mirrors.
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Wavelength effect on atomic and molecular high harmonic generation driven by a tunable infrared parametric source.
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Chemical physics: Electronic movies.
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Probing electron correlation via attosecond xuv pulses in the two-photon double ionization of helium.
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Generating single attosecond pulse using multi-cycle lasers in a polarization gate.
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A tabletop femtosecond time-resolved soft x-ray transient absorption spectrometer.
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Direct amplification of terawatt sub-10-fs pulses in a CPA system of Ti:sapphire laser.
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Generation of 0.5 mJ, few-cycle laser pulses by an adaptive phase modulator.
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Coherent water window x ray by phase-matched high-order harmonic generation in neutral media.
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Scaling of wave-packet dynamics in an intense midinfrared field.
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Attosecond light pulses for probing two-electron dynamics of helium in the time domain.
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Probe of high-order harmonic generation in a hollow waveguide geometry using counterpropagating light.
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Attosecond real-time observation of electron tunnelling in atoms.
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Single attosecond pulse generation from asymmetric molecules with a multicycle laser pulse.
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Molecular response properties from explicitly time-dependent configuration interaction methods.
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The future of attosecond spectroscopy.
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Attosecond control and measurement: lightwave electronics.
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Angle-resolved photoemission spectroscopy with a femtosecond high harmonic light source using a two-dimensional imaging electron analyzer.
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Dramatic enhancement of high-order harmonic generation.
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Bright multi-keV harmonic generation from relativistically oscillating plasma surfaces.
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Bright quasi-phase-matched soft-X-ray harmonic radiation from argon ions.
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Attosecond spectroscopy in condensed matter.
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Isolated attosecond pulses using a detuned second-harmonic field.
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Attosecond electron pulses for 4D diffraction and microscopy.
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Self-compression of attosecond high-order harmonic pulses.
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Spectral line shape variations in time-resolved photoemission from a solid.
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Quantum path interference in the wavelength dependence of high-harmonic generation.
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Conclusive evidence of an attosecond pulse train observed with the mode-resolved autocorrelation technique.
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Single attosecond pulse generation in the multicycle-driver regime by adding a weak second-harmonic field.
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Tomography of high harmonic generation in a cluster jet.
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Adaptive spatial control of fiber modes and their excitation for high-harmonic generation.
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Design, fabrication, and analysis of chirped multilayer mirrors for reflection of extreme-ultraviolet attosecond pulses.
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Direct interferometric measurement of the atomic dipole phase in high-order harmonic generation.
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Tunable ultrashort laser pulses generated through filamentation in gases.
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X-ray microprobe of orbital alignment in strong-field ionized atoms.
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Nonlinear optics of intense attosecond light pulses.
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Observation of relativistic cross-phase modulation in high-intensity laser-plasma interactions.
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Breaking resolution limits in ultrafast electron diffraction and microscopy.
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Relativistic attosecond electron pulses from a free-space laser-acceleration scheme.
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Generating single attosecond pulses via spatial filtering.
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Attosecond temporal gating with elliptically polarized light.
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Toward time-resolved soft X-ray microscopy using pulsed fs-high-harmonic radiation.
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Attosecond pulse extreme-ultraviolet photoionization in a two-color laser field.
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Compact, stable and efficient all-fibre gas cells using hollow-core photonic crystal fibres.
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Mapping attosecond electron wave packet motion.
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Probing molecular dynamics with attosecond resolution using correlated wave packet pairs.
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