Isotope selection in distance measurements between nitroxides

Jeschke G, Zimmermann H, Godt A (2006)
JOURNAL OF MAGNETIC RESONANCE 180(1): 137-146.

Download
Es wurde kein Volltext hochgeladen. Nur Publikationsnachweis!
Zeitschriftenaufsatz | Veröffentlicht | Englisch
Autor
; ;
Abstract / Bemerkung
Self-assembly of spin-labeled synthetic macromolecules or biomacrornolecules can lead to structures that contain more than two nitroxide radicals. Label-to-label distance distributions are then poorly resolved since established electron paramagnetic resonance techniques for distance measurements cannot select between the different pairs of nitroxides. A separation into different contributions can be achieved by partially labeling the nitroxide radicals by N-15 or by deuterium and applying pulse electron electron double resonance techniques. With N-15 labeling, strong suppression of either the N-14 or the N-15 contribution can be achieved by Suitable choices of the excitation bandwidths and frequencies of the observer subsequence and pump pulse and linear combination of data sets. With deuterium labeling, interactions between only the isotope-labeled nitroxides can be selected by a two-dimensional version of the four-pulse double electron electron resonance experiment. This selection is based on the deep electron spin echo envelope modulation of deuterated nitroxides. (c) 2006 Elsevier Inc. All rights reserved.
Erscheinungsjahr
Zeitschriftentitel
JOURNAL OF MAGNETIC RESONANCE
Band
180
Ausgabe
1
Seite(n)
137-146
ISSN
PUB-ID

Zitieren

Jeschke G, Zimmermann H, Godt A. Isotope selection in distance measurements between nitroxides. JOURNAL OF MAGNETIC RESONANCE. 2006;180(1):137-146.
Jeschke, G., Zimmermann, H., & Godt, A. (2006). Isotope selection in distance measurements between nitroxides. JOURNAL OF MAGNETIC RESONANCE, 180(1), 137-146. doi:10.1016/j.jmr.2006.02.002
Jeschke, G., Zimmermann, H., and Godt, A. (2006). Isotope selection in distance measurements between nitroxides. JOURNAL OF MAGNETIC RESONANCE 180, 137-146.
Jeschke, G., Zimmermann, H., & Godt, A., 2006. Isotope selection in distance measurements between nitroxides. JOURNAL OF MAGNETIC RESONANCE, 180(1), p 137-146.
G. Jeschke, H. Zimmermann, and A. Godt, “Isotope selection in distance measurements between nitroxides”, JOURNAL OF MAGNETIC RESONANCE, vol. 180, 2006, pp. 137-146.
Jeschke, G., Zimmermann, H., Godt, A.: Isotope selection in distance measurements between nitroxides. JOURNAL OF MAGNETIC RESONANCE. 180, 137-146 (2006).
Jeschke, G, Zimmermann, H, and Godt, Adelheid. “Isotope selection in distance measurements between nitroxides”. JOURNAL OF MAGNETIC RESONANCE 180.1 (2006): 137-146.

17 Zitationen in Europe PMC

Daten bereitgestellt von Europe PubMed Central.

Dynamical decoupling of nitroxides in o-terphenyl: a study of temperature, deuteration and concentration effects.
Soetbeer J, Hülsmann M, Godt A, Polyhach Y, Jeschke G., Phys Chem Chem Phys 20(3), 2018
PMID: 29261205
A Bis-Manganese(II)-DOTA Complex for Pulsed Dipolar Spectroscopy.
Demay-Drouhard P, Ching HY, Akhmetzyanov D, Guillot R, Tabares LC, Bertrand HC, Policar C., Chemphyschem 17(13), 2016
PMID: 27017296
Conformation and EPR characterization of rigid, 310 -helical peptides with TOAC spin labels: Models for short distances.
Shabestari MH, van Son M, Moretto A, Crisma M, Toniolo C, Huber M., Biopolymers 102(3), 2014
PMID: 24488683
New developments in spin labels for pulsed dipolar EPR.
Fielding AJ, Concilio MG, Heaven G, Hollas MA., Molecules 19(10), 2014
PMID: 25342554
Isotope effects in ESR spectroscopy.
Stößer R, Herrmann W., Molecules 18(6), 2013
PMID: 23749159
EPR relaxation-enhancement-based distance measurements on orthogonally spin-labeled T4-lysozyme.
Razzaghi S, Brooks EK, Bordignon E, Hubbell WL, Yulikov M, Jeschke G., Chembiochem 14(14), 2013
PMID: 23775845
DEER distance measurements on proteins.
Jeschke G., Annu Rev Phys Chem 63(), 2012
PMID: 22404592
Spectroscopic selection of distance measurements in a protein dimer with mixed nitroxide and Gd3+ spin labels.
Kaminker I, Yagi H, Huber T, Feintuch A, Otting G, Goldfarb D., Phys Chem Chem Phys 14(13), 2012
PMID: 22362220
Distance measurements in Au nanoparticles functionalized with nitroxide radicals and Gd(3+)-DTPA chelate complexes.
Yulikov M, Lueders P, Warsi MF, Chechik V, Jeschke G., Phys Chem Chem Phys 14(30), 2012
PMID: 22743649
High sensitivity and versatility of the DEER experiment on nitroxide radical pairs at Q-band frequencies.
Polyhach Y, Bordignon E, Tschaggelar R, Gandra S, Godt A, Jeschke G., Phys Chem Chem Phys 14(30), 2012
PMID: 22751953
Spin pair geometry revealed by high-field DEER in the presence of conformational distributions.
Polyhach Y, Godt A, Bauer C, Jeschke G., J Magn Reson 185(1), 2007
PMID: 17188008
Long-range distance determinations in biomacromolecules by EPR spectroscopy.
Schiemann O, Prisner TF., Q Rev Biophys 40(1), 2007
PMID: 17565764

28 References

Daten bereitgestellt von Europe PubMed Central.

Application of ELDOR in electron-spin echo for paramagnetic center space distributions in solids
Milov, Fiz. Tverd. Tela (Leningrad) 23(), 1981
Electron–electron double-resonance in electron-spin echo: model biradical systems and the sensitized photolysis of decalin
Milov, Chem. Phys. Lett. 110(), 1984
Selection of dipolar interaction by the 2+1 pulse train ESE
Kurshev, J. Magn. Reson. 81(), 1989
Multiple-quantum ESR and distance measurements
Borbat, Chem. Phys. Lett. 313(), 1999
Dead-time free measurement of dipole-dipole interactions between electron spins.
Pannier M, Veit S, Godt A, Jeschke G, Spiess HW., J. Magn. Reson. 142(2), 2000
PMID: 10648151
Dipolar spectroscopy and spin alignment in electron paramagnetic resonance
Jeschke, Chem. Phys. Lett. 331(), 2000
Sensitivity enhancement in pulse EPR distance measurements.
Jeschke G, Bender A, Paulsen H, Zimmermann H, Godt A., J. Magn. Reson. 169(1), 2004
PMID: 15183350

AUTHOR UNKNOWN, 2000
A new spin on protein dynamics.
Columbus L, Hubbell WL., Trends Biochem. Sci. 27(6), 2002
PMID: 12069788
Site directed spin labelling and pulsed dipolar electron paramagnetic resonance (double electron–electron resonance) of force activation in muscle
Fajer, J. Phys.: Condens. Mat. 17(), 2005
Pulsed electron double resonance (PELDOR) and its applications in free-radicals research
Milov, Appl. Magn. Reson. 15(), 1998
Determination of the nanostructure of polymer materials by electron paramagnetic resonance spectroscopy
Jeschke, Macromol. Rapid Commun. 23(), 2002
Direct conversion of EPR dipolar time evolution data to distance distributions.
Jeschke G, Koch A, Jonas U, Godt A., J. Magn. Reson. 155(1), 2002
PMID: 11945035
Data analysis procedures for pulse ELDOR measurements of broad distance distributions
Jeschke, Appl. Magn. Reson. 26(), 2004
Visualization of distance distribution from pulsed double electron–electron resonance data
Bowman, Appl. Magn. Reson. 26(), 2004
The determination of pair distance distributions by pulsed ESR using Tikhonov regularization.
Chiang YW, Borbat PP, Freed JH., J. Magn. Reson. 172(2), 2005
PMID: 15649755
Localization of the N-terminal domain in light-harvesting chlorophyll a/b protein by EPR measurements.
Jeschke G, Bender A, Schweikardt T, Panek G, Decker H, Paulsen H., J. Biol. Chem. 280(19), 2005
PMID: 15755729
Assessing oligomerization of membrane proteins by four-pulse DEER: pH-dependent dimerization of NhaA Na+/H+ antiporter of E. coli.
Hilger D, Jung H, Padan E, Wegener C, Vogel KP, Steinhoff HJ, Jeschke G., Biophys. J. 89(2), 2005
PMID: 15894644

Lesk, 2004
Distance measurements in the nanometer range by pulse EPR.
Jeschke G., Chemphyschem 3(11), 2002
PMID: 12503132
EPR probes with well-defined, long distances between two or three unpaired electrons
Godt A, Franzen C, Veit S, Enkelmann V V, Pannier M, Jeschke G., J. Org. Chem. 65(22), 2000
PMID: 11076617

AUTHOR UNKNOWN, 0
Double-quantum ESR and distance measurements
Borbat, 2000
Zero deadtime pulsed ESR by remote echo detection
Cho, Chem. Phys. Lett. 160(), 1989

Schweiger, 2001

Export

Markieren/ Markierung löschen
Markierte Publikationen

Open Data PUB

Web of Science

Dieser Datensatz im Web of Science®

Quellen

PMID: 16495097
PubMed | Europe PMC

Suchen in

Google Scholar