Catalytic oxidation of hydrocarbons over Co3O4 catalyst prepared by CVD
Tian Z, Bahlawane N, Qi F, Kohse-Höinghaus K (2009)
CATALYSIS COMMUNICATIONS 11(2): 118-122.
Zeitschriftenaufsatz
| Veröffentlicht | Englisch
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Abstract / Bemerkung
The total oxidation of C2H2, C3H6, C3H8, n-C4H8, n-C4H10 and i-C4H10 was studied in a monolithic flow reactor under temperature-programmed mode and highly diluted conditions. The non-catalytic combustion of the investigated hydrocarbons leads to a substantial formation of CO and traces of methane at intermediate temperatures. This drawback was suppressed upon the deposition of a thin layer of Co3O4 on the monolith and all investigated hydrocarbons tend to light off at 250-290 degrees C. The apparent activation energy was found to exhibit a linear correlation with the C-H bond dissociation energy, indicating that the C-H activation is still the rate-limiting step. (C) 2009 Elsevier B.V. All rights reserved.
Stichworte
Hydrocarbon;
deposition;
Apparent activation energy;
Chemical vapor;
Catalytic combustion;
Cobalt oxide;
Bond dissociation energy
Erscheinungsjahr
2009
Zeitschriftentitel
CATALYSIS COMMUNICATIONS
Band
11
Ausgabe
2
Seite(n)
118-122
ISSN
1566-7367
Page URI
https://pub.uni-bielefeld.de/record/1589608
Zitieren
Tian Z, Bahlawane N, Qi F, Kohse-Höinghaus K. Catalytic oxidation of hydrocarbons over Co3O4 catalyst prepared by CVD. CATALYSIS COMMUNICATIONS. 2009;11(2):118-122.
Tian, Z., Bahlawane, N., Qi, F., & Kohse-Höinghaus, K. (2009). Catalytic oxidation of hydrocarbons over Co3O4 catalyst prepared by CVD. CATALYSIS COMMUNICATIONS, 11(2), 118-122. https://doi.org/10.1016/j.catcom.2009.09.008
Tian, Zhenyu, Bahlawane, Naoufal, Qi, Fei, and Kohse-Höinghaus, Katharina. 2009. “Catalytic oxidation of hydrocarbons over Co3O4 catalyst prepared by CVD”. CATALYSIS COMMUNICATIONS 11 (2): 118-122.
Tian, Z., Bahlawane, N., Qi, F., and Kohse-Höinghaus, K. (2009). Catalytic oxidation of hydrocarbons over Co3O4 catalyst prepared by CVD. CATALYSIS COMMUNICATIONS 11, 118-122.
Tian, Z., et al., 2009. Catalytic oxidation of hydrocarbons over Co3O4 catalyst prepared by CVD. CATALYSIS COMMUNICATIONS, 11(2), p 118-122.
Z. Tian, et al., “Catalytic oxidation of hydrocarbons over Co3O4 catalyst prepared by CVD”, CATALYSIS COMMUNICATIONS, vol. 11, 2009, pp. 118-122.
Tian, Z., Bahlawane, N., Qi, F., Kohse-Höinghaus, K.: Catalytic oxidation of hydrocarbons over Co3O4 catalyst prepared by CVD. CATALYSIS COMMUNICATIONS. 11, 118-122 (2009).
Tian, Zhenyu, Bahlawane, Naoufal, Qi, Fei, and Kohse-Höinghaus, Katharina. “Catalytic oxidation of hydrocarbons over Co3O4 catalyst prepared by CVD”. CATALYSIS COMMUNICATIONS 11.2 (2009): 118-122.
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