Fast, flexible algorithm for calculating photon correlations

Laurence TA, Fore S, Huser T (2006)
Optics Letters 31(6): 829-831.

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Abstract
We introduce a new algorithm for computing correlations of photon arrival time data acquired in single-molecule fluorescence spectroscopy and fluorescence correlation spectroscopy (FCS). The algorithm is based on rewriting the correlation as a counting operation on photon pairs and can be used with arbitrary bin widths and spacing. The flexibility of the algorithm is demonstrated by use of FCS simulations and single-molecule photon antibunching experiments. Execution speed is comparable to the commonly used multiple-tau correlation technique. Wide bin spacings are possible that allow for real-time software calculation of correlations, even for high count rates. (c) 2006 Optical Society of America.
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Laurence TA, Fore S, Huser T. Fast, flexible algorithm for calculating photon correlations. Optics Letters. 2006;31(6):829-831.
Laurence, T. A., Fore, S., & Huser, T. (2006). Fast, flexible algorithm for calculating photon correlations. Optics Letters, 31(6), 829-831.
Laurence, T. A., Fore, S., and Huser, T. (2006). Fast, flexible algorithm for calculating photon correlations. Optics Letters 31, 829-831.
Laurence, T.A., Fore, S., & Huser, T., 2006. Fast, flexible algorithm for calculating photon correlations. Optics Letters, 31(6), p 829-831.
T.A. Laurence, S. Fore, and T. Huser, “Fast, flexible algorithm for calculating photon correlations”, Optics Letters, vol. 31, 2006, pp. 829-831.
Laurence, T.A., Fore, S., Huser, T.: Fast, flexible algorithm for calculating photon correlations. Optics Letters. 31, 829-831 (2006).
Laurence, T. A., Fore, S., and Huser, Thomas. “Fast, flexible algorithm for calculating photon correlations”. Optics Letters 31.6 (2006): 829-831.
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High-throughput FCS using an LCOS spatial light modulator and an 8 × 1 SPAD array.
Colyer RA, Scalia G, Rech I, Gulinatti A, Ghioni M, Cova S, Weiss S, Michalet X., Biomed Opt Express 1(5), 2010
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Single-quantum dot imaging with a photon counting camera.
Michalet X, Colyer RA, Antelman J, Siegmund OH, Tremsin A, Vallerga JV, Weiss S., Curr Pharm Biotechnol 10(5), 2009
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Real-time data acquisition incorporating high-speed software correlator for single-molecule spectroscopy.
Yang LL, Lee HY, Wang MK, Lin XY, Hsu KH, Chang YR, Fann W, White JD., J Microsc 234(3), 2009
PMID: 19493109
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Persson G, Sanden T, Sandberg A, Widengren J., Phys Chem Chem Phys 11(21), 2009
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PMID: 18303118
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PMID: 16844775

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