Coherent two-dimensional nanoscopy

Aeschlimann M, Brixner T, Fischer A, Kramer C, Melchior P, Pfeiffer W, Schneider C, Strüber C, Tuchscherer P, Voronine D (2011)
Science 333(6050): 1723-1726.

Download
No fulltext has been uploaded. References only!
Journal Article | Original Article | Published | English

No fulltext has been uploaded

Author
; ; ; ; ; ; ; ; ;
Abstract
We introduce a spectroscopic method that determines nonlinear quantum mechanical response functions beyond the optical diffraction limit and allows direct imaging of nanoscale coherence. In established coherent two-dimensional (2D) spectroscopy, four-wave–mixing responses are measured using three ingoing waves and one outgoing wave; thus, the method is diffraction-limited in spatial resolution. In coherent 2D nanoscopy, we use four ingoing waves and detect the final state via photoemission electron microscopy, which has 50-nanometer spatial resolution. We recorded local nanospectra from a corrugated silver surface and observed subwavelength 2D line shape variations. Plasmonic phase coherence of localized excitations persisted for about 100 femtoseconds and exhibited coherent beats. The observations are best explained by a model in which coupled oscillators lead to Fano-like resonances in the hybridized dark- and bright-mode response.
Publishing Year
ISSN
eISSN
PUB-ID

Cite this

Aeschlimann M, Brixner T, Fischer A, et al. Coherent two-dimensional nanoscopy. Science. 2011;333(6050):1723-1726.
Aeschlimann, M., Brixner, T., Fischer, A., Kramer, C., Melchior, P., Pfeiffer, W., Schneider, C., et al. (2011). Coherent two-dimensional nanoscopy. Science, 333(6050), 1723-1726. doi:10.1126/science.1209206
Aeschlimann, M., Brixner, T., Fischer, A., Kramer, C., Melchior, P., Pfeiffer, W., Schneider, C., Strüber, C., Tuchscherer, P., and Voronine, D. (2011). Coherent two-dimensional nanoscopy. Science 333, 1723-1726.
Aeschlimann, M., et al., 2011. Coherent two-dimensional nanoscopy. Science, 333(6050), p 1723-1726.
M. Aeschlimann, et al., “Coherent two-dimensional nanoscopy”, Science, vol. 333, 2011, pp. 1723-1726.
Aeschlimann, M., Brixner, T., Fischer, A., Kramer, C., Melchior, P., Pfeiffer, W., Schneider, C., Strüber, C., Tuchscherer, P., Voronine, D.: Coherent two-dimensional nanoscopy. Science. 333, 1723-1726 (2011).
Aeschlimann, M., Brixner, T., Fischer, A., Kramer, C., Melchior, P., Pfeiffer, Walter, Schneider, C., Strüber, Christian, Tuchscherer, P., and Voronine, Dmitri. “Coherent two-dimensional nanoscopy”. Science 333.6050 (2011): 1723-1726.
This data publication is cited in the following publications:
This publication cites the following data publications:

25 Citations in Europe PMC

Data provided by Europe PubMed Central.

Rapid-scan coherent 2D fluorescence spectroscopy.
Draeger S, Roeding S, Brixner T., Opt Express 25(4), 2017
PMID: 28241542
Optimizing sparse sampling for 2D electronic spectroscopy.
Roeding S, Klimovich N, Brixner T., J Chem Phys 146(8), 2017
PMID: 28249459
Incoherent population mixing contributions to phase-modulation two-dimensional coherent excitation spectra.
Grégoire P, Srimath Kandada AR, Vella E, Tao C, Leonelli R, Silva C., J Chem Phys 147(11), 2017
PMID: 28938824
Giant nonlinear response at a plasmonic nanofocus drives efficient four-wave mixing.
Nielsen MP, Shi X, Dichtl P, Maier SA, Oulton RF., Science 358(6367), 2017
PMID: 29191907
Ultrafast and nonlinear surface-enhanced Raman spectroscopy.
Gruenke NL, Cardinal MF, McAnally MO, Frontiera RR, Schatz GC, Van Duyne RP., Chem Soc Rev 45(8), 2016
PMID: 26848784
Attosecond nanoscale near-field sampling.
Förg B, Schötz J, Süßmann F, Förster M, Krüger M, Ahn B, Okell WA, Wintersperger K, Zherebtsov S, Guggenmos A, Pervak V, Kessel A, Trushin SA, Azzeer AM, Stockman MI, Kim D, Krausz F, Hommelhoff P, Kling MF., Nat Commun 7(), 2016
PMID: 27241851
Realistic Silver Optical Constants for Plasmonics.
Jiang Y, Pillai S, Green MA., Sci Rep 6(), 2016
PMID: 27470307
Suppressing sampling noise in linear and two-dimensional spectral simulations.
Kruiger JF, van der Vegte CP, Jansen TL., J Chem Phys 142(5), 2015
PMID: 25662638
Energy transfer pathways in semiconducting carbon nanotubes revealed using two-dimensional white-light spectroscopy.
Mehlenbacher RD, McDonough TJ, Grechko M, Wu MY, Arnold MS, Zanni MT., Nat Commun 6(), 2015
PMID: 25865487
Nanoscale Imaging of Local Few-Femtosecond Near-Field Dynamics within a Single Plasmonic Nanoantenna.
Mårsell E, Losquin A, Svärd R, Miranda M, Guo C, Harth A, Lorek E, Mauritsson J, Arnold CL, Xu H, L'Huillier A, Mikkelsen A., Nano Lett 15(10), 2015
PMID: 26375959
Ultrafast dynamics of single molecules.
Brinks D, Hildner R, van Dijk EM, Stefani FD, Nieder JB, Hernando J, van Hulst NF., Chem Soc Rev 43(8), 2014
PMID: 24473271
Shaping and spatiotemporal characterization of sub-10-fs pulses focused by a high-NA objective.
Pawłowska M, Goetz S, Dreher C, Wurdack M, Krauss E, Razinskas G, Geisler P, Hecht B, Brixner T., Opt Express 22(25), 2014
PMID: 25607100
Surface hopping modeling of two-dimensional spectra.
Tempelaar R, van der Vegte CP, Knoester J, Jansen TL., J Chem Phys 138(16), 2013
PMID: 23635110
Spectroscopic signatures of quantum-coherent energy transfer.
Collini E., Chem Soc Rev 42(12), 2013
PMID: 23417162
Molecular decision trees realized by ultrafast electronic spectroscopy.
Fresch B, Hiluf D, Collini E, Levine RD, Remacle F., Proc Natl Acad Sci U S A 110(43), 2013
PMID: 24043793
Plasmonic antennas as design elements for coherent ultrafast nanophotonics.
Brinks D, Castro-Lopez M, Hildner R, van Hulst NF., Proc Natl Acad Sci U S A 110(46), 2013
PMID: 24163355
Multidimensional coherent photocurrent spectroscopy of a semiconductor nanostructure.
Nardin G, Autry TM, Silverman KL, Cundiff ST., Opt Express 21(23), 2013
PMID: 24514373
Exciton transport in thin-film cyanine dye J-aggregates.
Valleau S, Saikin SK, Yung MH, Aspuru Guzik A., J Chem Phys 137(3), 2012
PMID: 22830685
Time-resolved surface-enhanced coherent sensing of nanoscale molecular complexes.
Voronine DV, Sinyukov AM, Hua X, Wang K, Jha PK, Munusamy E, Wheeler SE, Welch G, Sokolov AV, Scully MO., Sci Rep 2(), 2012
PMID: 23189240

26 References

Data provided by Europe PubMed Central.

Femtosecond polarization pulse shaping.
Brixner T, Gerber G., Opt Lett 26(8), 2001
PMID: 18040384

Export

0 Marked Publications

Open Data PUB

Web of Science

View record in Web of Science®

Sources

PMID: 21835982
PubMed | Europe PMC

Search this title in

Google Scholar