Energy transfer in combustion diagnostics: Experiment and modeling

Brockhinke A, Kohse-Höinghaus K (2001)
FARADAY DISCUSSIONS 119(1): 275-286.

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Zeitschriftenaufsatz | Veröffentlicht | Englisch
Abstract / Bemerkung
Laser induced fluorescence (LIF) of OH (A (2)Sigma (+)) is measured in several atmospheric-pressure flames using a short-pulse laser system (80 ps duration) in conjunction with an intensified streak camera. The two-dimensional signal-detection technique allows one to simultaneously monitor rotational and vibrational relaxation as well as electronic quenching. Rotationally-resolved LIF spectra affected by energy transfer are compared with the results of a rate-equation model and are found to be in reasonably good agreement. It is shown that a significant contribution of fluorescence detected by broad-band techniques is due to levels populated by vibrational energy transfer (VET). Implications for picosecond LIF techniques for the time-resolved, quench-free detection of OH are discussed. A detailed analysis is presented for fluorescence spectra originating from levels populated by VET after excitation of states in the OH (A (2)Sigma (+), v' = 2) level.
Erscheinungsjahr
Zeitschriftentitel
FARADAY DISCUSSIONS
Band
119
Zeitschriftennummer
1
Seite
275-286
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eISSN
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Brockhinke A, Kohse-Höinghaus K. Energy transfer in combustion diagnostics: Experiment and modeling. FARADAY DISCUSSIONS. 2001;119(1):275-286.
Brockhinke, A., & Kohse-Höinghaus, K. (2001). Energy transfer in combustion diagnostics: Experiment and modeling. FARADAY DISCUSSIONS, 119(1), 275-286. doi:10.1039/b102058g
Brockhinke, A., and Kohse-Höinghaus, K. (2001). Energy transfer in combustion diagnostics: Experiment and modeling. FARADAY DISCUSSIONS 119, 275-286.
Brockhinke, A., & Kohse-Höinghaus, K., 2001. Energy transfer in combustion diagnostics: Experiment and modeling. FARADAY DISCUSSIONS, 119(1), p 275-286.
A. Brockhinke and K. Kohse-Höinghaus, “Energy transfer in combustion diagnostics: Experiment and modeling”, FARADAY DISCUSSIONS, vol. 119, 2001, pp. 275-286.
Brockhinke, A., Kohse-Höinghaus, K.: Energy transfer in combustion diagnostics: Experiment and modeling. FARADAY DISCUSSIONS. 119, 275-286 (2001).
Brockhinke, Andreas, and Kohse-Höinghaus, Katharina. “Energy transfer in combustion diagnostics: Experiment and modeling”. FARADAY DISCUSSIONS 119.1 (2001): 275-286.

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PMID: 11877996
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