Attosecond real-time observation of electron tunnelling in atoms

Uiberacker M, Uphues T, Schultze M, Verhoef AJ, Yakovlev V, Kling MF, Rauschenberger J, Kabachnik NM, Schröder H, Lezius M, Kompa KL, et al. (2007)
Nature 446(7136): 627-632.

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Atoms exposed to intense light lose one or more electrons and become ions. In strong fields, the process is predicted to occur via tunnelling through the binding potential that is suppressed by the light field near the peaks of its oscillations. Here we report the real-time observation of this most elementary step in strong-field interactions: light-induced electron tunnelling. The process is found to deplete atomic bound states in sharp steps lasting several hundred attoseconds. This suggests a new technique, attosecond tunnelling, for probing short-lived, transient states of atoms or molecules with high temporal resolution. The utility of attosecond tunnelling is demonstrated by capturing multi-electron excitation (shake-up) and relaxation ( cascaded Auger decay) processes with subfemtosecond resolution.
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Uiberacker M, Uphues T, Schultze M, et al. Attosecond real-time observation of electron tunnelling in atoms. Nature. 2007;446(7136):627-632.
Uiberacker, M., Uphues, T., Schultze, M., Verhoef, A. J., Yakovlev, V., Kling, M. F., Rauschenberger, J., et al. (2007). Attosecond real-time observation of electron tunnelling in atoms. Nature, 446(7136), 627-632. doi:10.1038/nature05648
Uiberacker, M., Uphues, T., Schultze, M., Verhoef, A. J., Yakovlev, V., Kling, M. F., Rauschenberger, J., Kabachnik, N. M., Schröder, H., Lezius, M., et al. (2007). Attosecond real-time observation of electron tunnelling in atoms. Nature 446, 627-632.
Uiberacker, M., et al., 2007. Attosecond real-time observation of electron tunnelling in atoms. Nature, 446(7136), p 627-632.
M. Uiberacker, et al., “Attosecond real-time observation of electron tunnelling in atoms”, Nature, vol. 446, 2007, pp. 627-632.
Uiberacker, M., Uphues, T., Schultze, M., Verhoef, A.J., Yakovlev, V., Kling, M.F., Rauschenberger, J., Kabachnik, N.M., Schröder, H., Lezius, M., Kompa, K.L., Muller, H.-G., Vrakking, M.J.J., Hendel, S., Kleineberg, U., Heinzmann, U., Drescher, M., Krausz, F.: Attosecond real-time observation of electron tunnelling in atoms. Nature. 446, 627-632 (2007).
Uiberacker, M., Uphues, Thorsten, Schultze, M., Verhoef, A. J., Yakovlev, V., Kling, M. F., Rauschenberger, J., Kabachnik, Nikolay M., Schröder, H., Lezius, M., Kompa, K. L., Muller, H. -G., Vrakking, M. J. J., Hendel, Stefan, Kleineberg, U., Heinzmann, Ulrich, Drescher, Markus, and Krausz, F. “Attosecond real-time observation of electron tunnelling in atoms”. Nature 446.7136 (2007): 627-632.
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88 Citations in Europe PMC

Data provided by Europe PubMed Central.

Attosecond electron dynamics.
Kling MF, Vrakking MJ., Annu Rev Phys Chem 59(), 2008
PMID: 18031218
Single-cycle nonlinear optics.
Goulielmakis E, Schultze M, Hofstetter M, Yakovlev VS, Gagnon J, Uiberacker M, Aquila AL, Gullikson EM, Attwood DT, Kienberger R, Krausz F, Kleineberg U., Science 320(5883), 2008
PMID: 18566281
A tabletop femtosecond time-resolved soft x-ray transient absorption spectrometer.
Loh ZH, Khalil M, Correa RE, Leone SR., Rev Sci Instrum 79(7), 2008
PMID: 18681685
Attophysics: tunnel vision.
Marangos JP., Nature 446(7136), 2007
PMID: 17410163
Attosecond control and measurement: lightwave electronics.
Goulielmakis E, Yakovlev VS, Cavalieri AL, Uiberacker M, Pervak V, Apolonski A, Kienberger R, Kleineberg U, Krausz F., Science 317(5839), 2007
PMID: 17690286
Soft X-ray-driven femtosecond molecular dynamics.
Gagnon E, Ranitovic P, Tong XM, Cocke CL, Murnane MM, Kapteyn HC, Sandhu AS., Science 317(5843), 2007
PMID: 17823349
Attophysics: at a glance.
Villeneuve DM., Nature 449(7165), 2007
PMID: 17960231
Attosecond resolved charging of ions in a rare-gas cluster.
Georgescu I, Saalmann U, Rost JM., Phys Rev Lett 99(18), 2007
PMID: 17995403
Generation and photonic guidance of multi-octave optical-frequency combs.
Couny F, Benabid F, Roberts PJ, Light PS, Raymer MG., Science 318(5853), 2007
PMID: 18006741
Attosecond electron pulses for 4D diffraction and microscopy.
Baum P, Zewail AH., Proc Natl Acad Sci U S A 104(47), 2007
PMID: 18000040
Attosecond control of ionization by wave-packet interference.
Johnsson P, Mauritsson J, Remetter T, L'Huillier A, Schafer KJ., Phys Rev Lett 99(23), 2007
PMID: 18233360

28 References

Data provided by Europe PubMed Central.

Auger cascades versus direct double Auger: relaxation processes following photoionization of the Kr 3d and Xe 4d, 3d inner shells
Viefhaus, Journal of Physics B Atomic Molecular and Optical Physics 38(21), 2005
Coulomb and polarization effects in laser-assisted XUV ionization
Smirnova, Journal of Physics B Atomic Molecular and Optical Physics 39(13), 2006
Isolated single-cycle attosecond pulses.
Sansone G, Benedetti E, Calegari F, Vozzi C, Avaldi L, Flammini R, Poletto L, Villoresi P, Altucci C, Velotta R, Stagira S, De Silvestri S, Nisoli M., Science 314(5798), 2006
PMID: 17053142

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