Single-active-electron ionization of C-60 in intense laser pulses to high charge states

Jaron-Becker A, Becker A, Faisal F (2007)
JOURNAL OF CHEMICAL PHYSICS 126(12).

Journal Article | Published | English

No fulltext has been uploaded

Author
; ;
Abstract
Sequential ionization of the C-60 fullerene to high charge states in ultrashort intense laser pulses is investigated within the strong-field S-matrix approach. Ion yields are calculated and saturation intensities are determined for a broad range of laser wavelengths between 395 and 1800 nm at different pulse lengths. Comparisons of the S-matrix predictions for the saturation intensities with recent experimental data are in an overall satisfactory agreement, indicating that saturation of ionization of this complex molecule can be well described using the single-active-electron approach. The analysis of the results shows that the contributions from the h(u)-highest occupied molecular orbital to the ion yields dominate as compared to those from the inner valence shells h(g) and g(g). Finally, it is demonstrated that the suppression of ionization of C-60 and its ions, as observed in experiments, can be interpreted within the present theory as due to the finite cage size of the fullerenes and a multi-slit-like interference effect between partial waves emitted from the different nuclei of the fullerenes. (c) 2007 American Institute of Physics.
Publishing Year
ISSN
PUB-ID

Cite this

Jaron-Becker A, Becker A, Faisal F. Single-active-electron ionization of C-60 in intense laser pulses to high charge states. JOURNAL OF CHEMICAL PHYSICS. 2007;126(12).
Jaron-Becker, A., Becker, A., & Faisal, F. (2007). Single-active-electron ionization of C-60 in intense laser pulses to high charge states. JOURNAL OF CHEMICAL PHYSICS, 126(12).
Jaron-Becker, A., Becker, A., and Faisal, F. (2007). Single-active-electron ionization of C-60 in intense laser pulses to high charge states. JOURNAL OF CHEMICAL PHYSICS 126.
Jaron-Becker, A., Becker, A., & Faisal, F., 2007. Single-active-electron ionization of C-60 in intense laser pulses to high charge states. JOURNAL OF CHEMICAL PHYSICS, 126(12).
A. Jaron-Becker, A. Becker, and F. Faisal, “Single-active-electron ionization of C-60 in intense laser pulses to high charge states”, JOURNAL OF CHEMICAL PHYSICS, vol. 126, 2007.
Jaron-Becker, A., Becker, A., Faisal, F.: Single-active-electron ionization of C-60 in intense laser pulses to high charge states. JOURNAL OF CHEMICAL PHYSICS. 126, (2007).
Jaron-Becker, A., Becker, A., and Faisal, Farhard. “Single-active-electron ionization of C-60 in intense laser pulses to high charge states”. JOURNAL OF CHEMICAL PHYSICS 126.12 (2007).
This data publication is cited in the following publications:
This publication cites the following data publications:

3 Citations in Europe PMC

Data provided by Europe PubMed Central.

Fragmentation and ionization dynamics of C60 in elliptically polarized femtosecond laser fields.
Hertel IV, Shchatsinin I, Laarmann T, Zhavoronkov N, Ritze HH, Schulz CP., Phys. Rev. Lett. 102(2), 2009
PMID: 19257268
Ultrafast energy redistribution in C(60) fullerenes: a real time study by two-color femtosecond spectroscopy.
Shchatsinin I, Laarmann T, Zhavoronkov N, Schulz CP, Hertel IV., J Chem Phys 129(20), 2008
PMID: 19045865

68 References

Data provided by Europe PubMed Central.


AUTHOR UNKNOWN, 0
Coulomb stability limit of highly charged Cq+60 fullerenes.
Diaz-Tendero S, Alcami M, Martin F., Phys. Rev. Lett. 95(1), 2005
PMID: 16090614

Sahnoun, Chem Phys Lett 430(), 2006
Theoretical investigation of the stability of highly charged C60 molecules produced with intense near-infrared laser pulses.
Sahnoun R, Nakai K, Sato Y, Kono H, Fujimura Y, Tanaka M., J Chem Phys 125(18), 2006
PMID: 17115751

AUTHOR UNKNOWN, 0

AUTHOR UNKNOWN, 0

AUTHOR UNKNOWN, 0
Suppressed molecular ionization for a class of diatomics in intense femtosecond laser fields
Muth-Bohm J, Becker A, Faisal FH., Phys. Rev. Lett. 85(11), 2000
PMID: 10977991

AUTHOR UNKNOWN, 0

AUTHOR UNKNOWN, 0

AUTHOR UNKNOWN, 0

Chin, Can J Phys 48(), 1970

AUTHOR UNKNOWN, 0

AUTHOR UNKNOWN, 0

AUTHOR UNKNOWN, 0

AUTHOR UNKNOWN, 0

AUTHOR UNKNOWN, 0

AUTHOR UNKNOWN, 0

Export

0 Marked Publications

Open Data PUB

Web of Science

View record in Web of Science®

Sources

PMID: 17411126
PubMed | Europe PMC

Search this title in

Google Scholar